Radioactive Waste Streams: Waste Classification for Disposal
Congressional research reportDec 13, 2006
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Radioactive Waste Streams: Waste
Classification for Disposal
-name redactedSpecialist in Energy and Energy Infrastructure Policy
December 13, 2006
Congressional Research Service
7-....
www.crs.gov
RL32163
CRS Report for Congress
Prepared for Members and Committees of Congress
Radioactive Waste Streams: Waste Classification for Disposal
Summary
Radioactive waste is a byproduct of nuclear weapons production, commercial nuclear power
generation, and the naval reactor program. Waste byproducts also result from radioisotopes used
for scientific, medical, and industrial purposes. The legislative definitions adopted for radioactive
wastes, for the most part, refer to the processes that generated the wastes. Thus, waste disposal
policies have tended to link the processes to uniquely tailored disposal solutions. Consequently,
the origin of the waste, rather than its radiologic characteristics, often determines its fate.
Plutonium and enriched uranium-235 were first produced by the Manhattan Project during World
War II. These materials were later defined by the Atomic Energy Act of 1954 as special nuclear
materials, along with other materials that the former Atomic Energy Commission (AEC)
determined were capable of releasing energy through nuclear fission. Reprocessing of irradiated
nuclear fuel to extract special nuclear material generated highly radioactive liquid and solid
byproducts. The Nuclear Waste Policy Act of 1982 (NWPA) defined irradiated fuel as spent
nuclear fuel, and the byproducts as high-level waste. Uranium ore processing technologically
enhanced naturally occurring radioactive material and left behind uranium mill tailings. The
fabrication of nuclear weapons generated transuranic waste. Both commercial and naval reactors
continue to generate spent fuel. High-level waste generation has ceased in the United States, as
irradiated fuel is no longer reprocessed. The routine operation and maintenance of nuclear
reactors, however, continues to generate low-level radioactive waste, as do medical procedures
using radioactive isotopes.
The NWPA provides for the permanent disposal of spent nuclear fuel and high-level radioactive
waste in a deep geologic repository. The repository is to be constructed and operated by the
Department of Energy (DOE) under the Nuclear Regulatory Commission’s (NRC) licensing
authority. Yucca Mountain, in Nevada, is the candidate site for the nation’s first repository.
The NRC and the Environmental Protection Agency (EPA) share regulatory authority for
radioactive waste disposal. However, these regulatory agencies have yet to adopt uniform
radiation protection standards for disposal sites. The NRC’s jurisdiction, however, does not
extend to DOE’s management of defense-related waste at DOE facilities other than Yucca
Mountain.
Radioactive waste classification continues to raise issues for policymakers. Most recently, DOE
policy on managing the residue in high-level waste storage tanks proved controversial enough
that Congress amended the definition of high-level waste. The disposition of waste with
characteristics left undefined by statute can be decided by an NRC administrative ruling. The case
for low-activity waste promises to provoke similar controversy. This report will be updated as
new radioactive waste classification issues arise.
Congressional Research Service
Radioactive Waste Streams: Waste Classification for Disposal
Contents
Background ................................................................................................................................1
Measurement of Radioactivity and Hazards of Radiation.............................................................2
Comparative Range of Radioactivity ...........................................................................................3
Spent Nuclear Fuel......................................................................................................................6
High-Level Radioactive Waste .................................................................................................. 12
Waste Incidental to Reprocessing .............................................................................................. 13
Transuranic Waste..................................................................................................................... 14
Surplus Weapons-Usable Plutonium.......................................................................................... 16
Low-Level Radioactive Waste................................................................................................... 16
Provisions for State Disposal Compacts............................................................................... 19
Low-Level Waste Classification Tables ............................................................................... 19
Mixed Low-Level Radioactive and Hazardous Waste ................................................................ 23
Depleted Uranium..................................................................................................................... 23
Technologically Enhanced Naturally Occurring Radioactive Material........................................ 24
Energy Policy Act Provisions for NORM ............................................................................ 25
Uranium Mill Tailings ............................................................................................................... 27
Waste Disposal Policy Issues..................................................................................................... 27
Glossary.................................................................................................................................... 29
Figures
Figure 1. Comparison of Radioactive Wastes...............................................................................4
Figure 2. Federal Sites, Commercial Reactor Storage Pools, and Independent Spent Fuel
Storage Installations .................................................................................................................8
Figure 3. Low-Level Waste Classification by Long-Lived Radionuclides................................... 20
Figure 4. Low-Level Waste Classification by Transuranic Radionuclides................................... 21
Figure 5. Low-Level Waste Classification by Short-Lived Radionuclides .................................. 21
Figure 6. Low-Level Waste Classification by Mixed Long-Lived and Short-Lived
Radionuclides ........................................................................................................................ 22
Figure A-1. 10 CFR 61.55 Table 1............................................................................................. 33
Figure A-2. 10 CFR 61.55 Table 2............................................................................................. 33
Tables
Table 1. Contribution to Average Annual Exposures from Natural and Artificial
Radioactive Sources.................................................................................................................3
Table 2. Legislative and Regulatory Reference to Waste Definitions ............................................5
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Radioactive Waste Streams: Waste Classification for Disposal
Table 3. Federal Site, Commercial Reactor Pool, and Independent Spent Fuel Storage.................9
Table 4. Physical Form and Characteristics of Low-Level Waste ............................................... 18
Table A-1. Uranium Mill Tailing Site Volume and Activity ........................................................ 31
Table A-2. Low-Level Waste Commercial Disposal Site Volume and Activity............................ 31
Table A-3. Spent Fuel Specific Activity ..................................................................................... 31
Appendixes
Appendix. ................................................................................................................................ 31
Contacts
Author Contact Information ...................................................................................................... 34
Congressional Research Service
Radioactive Waste Streams: Waste Classification for Disposal
Background
Radioactive waste is a byproduct of nuclear weapons production, commercial nuclear power
generation, and the naval reactor program. Waste byproducts also result from radioisotopes used
for scientific, medical, and industrial purposes. Waste classification policies have tended to link
the processes that generate the waste to uniquely tailored disposal solutions. Consequently, the
origin of the waste, rather than its radiologic characteristics, often determines its fate.
Congress recently renewed its interest in radioactive waste classification when a Department of
Energy (DOE) order regarding the disposition of high-level waste storage tank residue was
legally challenged. As a result, Congress amended the statutory definition of high-level waste to
exclude such residue. 1 The classification of other radioactive wastes continues to remain an
aspect of disposal policy.
The Atomic Energy Act of 1946 (P.L. 79-585) defined fissionable materials to include plutonium,
uranium-235, and other materials that the Atomic Energy Commission (AEC) determined to be
capable of releasing substantial quantities of energy through nuclear fission. Source material
included any uranium, thorium, or beryllium containing ore essential to producing fissionable
material, and byproduct material remaining after the fissionable material’s production. In the
amended Atomic Energy Act of 1954 (P.L. 83-703), the term special nuclear material superseded
fissionable material and included uranium enriched in isotope 233, material the AEC determined
to be special nuclear material, or any artificially enriched material.2
As the exclusive producer, the AEC originally retained title to all fissionable material for national
security reasons. In the 1954 amended Act, Congress authorized the AEC to license commercial
reactors, and ease restrictions on private companies using special nuclear material. Section 183
(Terms of Licenses) of the Act, however, kept government title to all special nuclear material
utilized or produced by the licensed facilities in the United States. In 1964, the AEC was
authorized to issue commercial licenses to possess special nuclear material subject to specific
licensing conditions (P.L. 88-489).
Although the Atomic Energy Act referred to transuranic waste (material contaminated with
elements in atomic number greater than uranium), radioactive waste was not defined by statute
until the 1980s. High-level waste and spent nuclear fuel were defined by the Nuclear Waste
Policy Act (NWPA) of 1982 (42 U.S.C. 10101). Spent nuclear fuel is the highly radioactive fuel
rods withdrawn from nuclear reactors. High-level waste refers to the byproduct of reprocessing
irradiated fuel to remove plutonium and uranium. Low-level radioactive waste was defined by the
Low-Level Radioactive Waste Policy Act of 1980 (P.L. 95-573) as radioactive material that is not
high-level radioactive waste, spent nuclear fuel, or byproduct material, and radioactive material
that the Nuclear Regulatory Commission (NRC) classifies as low-level radioactive waste
consistent with existing law.
1
Section 3116 (Defense Site Acceleration Completion), Ronald W. Reagan Defense Authorization Act of FY2005
(P.L. 108-375).
2
Laws of 83rd Congress, 2nd Session, 1118-21.
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Radioactive Waste Streams: Waste Classification for Disposal
Measurement of Radioactivity and Hazards of
Radiation
The measurement of radioactivity and the hazards of radiation are, in themselves, complex
subjects. A discussion of radioactive waste would be incomplete without reference to some basic
terms and concepts.
Radioactive elements decay over time. The process of radioactive decay transforms an atom to
more a stable element through the release of radiation—alpha particles (two protons and two
neutrons), charged beta particles (positive or negative electrons), or gamma rays (electromagnetic
radiation).
Radioactivity is expressed in units of curies—the equivalent of 37 billion (37 x 109) atoms
disintegrating per second. The rate of radioactive decay is expressed as half-life—the time it takes
for half the atoms in a given amount of radioactive material to disintegrate. Radioactive elements
with shorter half-lives therefore decay more quickly.
The term for the absorption of radiation by living organisms is dose. The United States uses the
Roentgen Equivalent Man (rem) as the unit of equivalent dose in humans. Rem relates the
absorbed dose in human tissue to the effective biological damage of the radiation. 3 Not all
radiation has the same biological effect, even for the same amount of absorbed dose, as some
forms of radiation are more efficient than others in transferring their energy to living cells.
In 1977, the International Commission on Radiation Protection (ICRP) concluded that an
individual’s mortality risk factor from radiation-induced cancers was about 1 x10-4 from an
exposure of one rem dose (one lifetime chance out of 10,000 for developing fatal cancer per rem),
and recommended that members of the public should not receive annual exposures exceeding 500
millirem. 4 The exposure limit is made up of all sources of ionizing radiation that an individual
might be exposed to annually, which includes natural background and artificial radiation. An
individual in the United States receives an average annual effective dose equivalent to 360
millirem, as shown in Table 1.
3
Rem is the product of the dose measured in units of rad (100 ergs/gram) multiplied by a quality factor (Q) for each
type of radiation; that is rem = rad x Q. For gamma rays, Q = 1, thus the absorbed dose in rads equals rems. For
neutrons Q = 5, and alpha particles Q = 20; thus an absorbed dose of 1 rad is equivalent to 5 rem and 20 rem
respectively.
4
Recommendations of the International Commission on Radiological Protection, January 1977 (superseded by ICRP
60) (supersedes ICRP 1, 6 & 9).
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Radioactive Waste Streams: Waste Classification for Disposal
Table 1. Contribution to Average Annual Exposures from Natural and Artificial
Radioactive Sources
Contributor
millirem
Natural - Radon
200
Natural background radiation
100
Occupational related exposure
0.9
Consumer products excluding tobacco
13
Miscellaneous environmental sources
0.06
Medical - diagnostic x rays
39
Medical - nuclear medicine
14
Average Annual Effective
360
Source: National Council on Radiation Protection and Measurements, Report No. 9, Ionizing Radiation Exposure
of the Population of the United States, September 1, 1987.
The ICRP revised its conclusion on risk factors in 1990, and recommended that the annual limit
for effective dose be reduced to 100 millirem. 5 This limit is equivalent to natural background
radiation exclusive of radon. ICRP qualified the recommendation with data showing that even at a
continued exposure of 500 millirem, the change in age-specific mortality rate is very small—less
than 4.5% for females, less than 2.5% for males older than 50 years, and even less for males
under age 50.
The radiation protection standards for NRC activities licensed under 10 C.F.R. Part 206 are based
on a radiation dose limit of 100 millirem, excluding contributions from background radiation and
medical procedures. Unlike the NRC’s dose-based approach to acceptable hazard level, the
Environmental Protection Agency (EPA) uses a risk-based approach that relies on the “linear, nothreshold” model of low-level radiation effects. In the EPA model, risk is extrapolated as a
straight line from the high-dose exposure for Hiroshima and Nagasaki atomic bomb survivors
down to zero radiation exposure. Thus, the EPA model attributes risk to natural background levels
of radiation. For illustrative purposes, EPA considers a 1-in-10,000 risk that an individual will
develop cancer to be excessive, and has set a goal of 1-in-a- million risk in cleanup of chemically
contaminated sites. The Government Accountability Office (GAO) has concluded that the lowlevel radiation protection standards administered by EPA and NRC do not have a conclusive
scientific basis, as evidence of the effects of low-level radiation is lacking.7
Comparative Range of Radioactivity
The comparative range in radioactivity of various wastes and materials is presented in Figure 1.
Radioactivity is typically expressed in terms of “curies/ gram” for soil-like materials as well as
radioactive materials that are homogeneous in nature. However, because the inventories of some
5
International Commission on Radiation Protection, Recommendation of the International Commission on Radiation
Protection—Publication 60, Paragraph 161, 1990.
6
Part 20—Standards for Protection Against Radiation.
7
U.S. Government Accounting Office, Radiation Standards—Scientific Basis Inconclusive, and EPA and NRC
Disagreement Continues (GAO/RCED-00-152), June 2000.
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Radioactive Waste Streams: Waste Classification for Disposal
radioactive wastes are tracked in terms of “curies/cubic-meter,” that unit of measure has been
used here.
The lowest end of the scale (at the bottom of the figure) is represented by soils of the United
States—the source of natural background radiation. Radioactivity ranging from 3 to 40
microcuries/cubic-meter may be attributed to potassium, thorium and uranium in soils.
Phosphogypsum mining waste is the byproduct of ore processing that “technologically enhanced
naturally occurring radioactive material” (uranium) at higher levels than natural background (thus
the term—TENORM), and may range from 6.5 to 45 microcuries/cubic-meter. Uranium mill
tailings (referred to as 11e.(2) byproduct material) range from 97 to 750 microcuries/cubic-meter
at various sites (Appendix, Table A-1). On average, low-level waste ranges from 6.7 to 20
curies/cubic-meter based on the inventory of disposal facilities (Appendix, Table A-2); a lower
limit is left undefined by regulation, but an upper limit is set at 7,000 curies/cubic-meter based on
specific constituents. Transuranic waste ranges between from 47 to 147 curies/cubic-meter based
on the Waste Isolation Pilot Plant inventory. The vitrified high-level waste processed by the
Savannah River Site ranges from 6,700 to 250,000 curies/cubic-meter. Finally, spent fuel aged 10
to 100 years would range from 105,000 to 2.7 million curies/cubic-meter (Appendix, Table A-3).
These comparisons are for illustrative purposes only, as the radioactive constituents among the
examples are different.
Figure 1. Comparison of Radioactive Wastes
Notes:
Spent Fuel – BWR and PWR fuel rod assemblies 10 to 100 years decay time. Upper range of 2.67 x 106 for 14
year BWR to lower range of 1.05 x 105 for 100 year PWR. Source: Table A-13 of Appendix A to Yuaa Mt. EIS,
and Appendix C to “Investigation of Nuclide Importance to Functional Requirements Related to Transport and
Long-Term Storage of LWR Spent Fuel” (ORNL/TM/12742 – 1995).
High-level waste – Savannah River Site Vitrified HLW. Source: Personal Communication with W. Pearson,
USDOE Savannah River.
Transuranic waste – 47 Ci/m3 for contact handled-TRU, 143 Ci/m3 for remote handled-TRU. Source: Table
1. of “The Waste Isolation Pilot Plant,” National Research Council (1996).
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Radioactive Waste Streams: Waste Classification for Disposal
Low-level waste – Average based on Table 1 of “Commercial Gross Volume and Activity Distribution in
Disposal of Low-Level and Mixed Low-Level Radioactive Waste During 1990” (DOE/EH-0332p, August 1993).
Upper and lower limits of SR-90 Table 2 of 10 CFR 61.55.
Uranium tailings – (11e.(2) byproduct material) ranges from 9.72x10-5 Ci/m3 at Maybell Mill Site Moffat
County, Co. to 7.48x10-4 at Salt Lake City Mill Site, Salt Lake County, UT. Source: Summary Table of
“Remediation of UMTRCA Title I Uranium Mill Sites Under the UMTRCA Project.” EIA (December 31, 1999).
http://www.eia.doe.gov/cneaf/nuclear/page/umtra/title1sum.html.
Phosphogypsum waste – (Technologically Enhanced Naturally Occurring Radioactive Material) Calculated
average of 6.5 to 45x10-6 Ci/m3 based on 7.3 to 36.7 x 10-12 Ci/g. Source: Summary Table. U.S. EPA TENORM.
http://www.epa.gov/radiation/tenorm/sources_table.htm and density range of 888 to 1130 kg/m3 for Type 65
Florida phosphogypsum, http://www.agrium.com/1342.cfm.
Soils of the U.S. – Range from 3 to 40 x 10-6 Ci/m3. Source: Personal communication with J.K. Otton, USGS.
Definitions of various radioactive wastes are summarized in Table 2 along with applicable
legislative provisions. More detailed descriptions of the wastes and the processes that generate the
wastes are provided further below.
Table 2. Legislative and Regulatory Reference to Waste Definitions
Definition
Reference
Spent Nuclear Fuel (SNF) . . . withdrawn from a nuclear
reactor following irradiation
Nuclear Waste Policy Act of 1982, 42 U.S.C. 10101
High-Level Waste (HLW) . . . highly radioactive material from
reprocessing spent nuclear fuel
Nuclear Waste Policy Act of 1982, 42 U.S.C. 10101
Radioactive Waste Incidental to Reprocessing . . . reclassified
waste stream that would otherwise be considered highlevel due to its source or concentration
Defense Authorization Act for Fiscal Year 2005, P.L.
108-375
Transuranic Waste (TRU) . . . man-made elements above
atomic number 92
Atomic Energy Act of 1954, 42 U.S.C. 2014
Surplus Weapons-Usable Plutonium
Non-Proliferation and Export Control Policy,
PDD/NSC 13 1993
Low-Level Radioactive Waste (LLRW) . . . not high-level
radioactive waste, spent nuclear fuel, transuranic waste, or
by-product material
Low-Level Radioactive Waste Policy Amendments Act
of 1985, P.L. 99-240
Class A, Class B, Class C Waste
Greater than Class C (GTCC)
Licensing Requirements for Land Disposal of
Radioactive Waste, 10 C.F.R. 61.55
Mixed Low Level Radioactive and Hazardous Waste . . . lowlevel radioactive waste under LLRWA and hazardous
chemicals regulated under RCRA
Low-Level Radioactive Waste Policy Act of 1985—42
U.S.C. 2021b & Resource Conservation and Recovery
Act of 1976—42 U.S.C. 6901
Uranium Mill Tailings . . . by-product material . . . naturally
occurring radioactive material and uranium ore mill tailings
Uranium Mill Tailings Radiation Control Act of
1978—42 U.S.C. 7901
Depleted Uranium Hexafluoride . . . the source material
uranium in which the isotope U-235 is less than 0.711
percent of the total uranium present
10 C.F.R. 40.4—Domestic Licensing of Source Material
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Radioactive Waste Streams: Waste Classification for Disposal
Spent Nuclear Fuel
Currently, 104 commercial nuclear power reactors are licensed by the NRC to operate in 31
states.8 These reactors are refueled on a frequency of 12 to 24 months. A generic Westinghousedesigned 1,000-megawatt pressurized-water reactor (PWR) operates with 100 metric tons of
nuclear fuel. During refueling, approximately one-third of the fuel (spent nuclear fuel) is
replaced. The spent fuel is moved to a storage pool adjacent to the reactor for thermal cooling and
decay of short-lived radionuclides.
Due to the limited storage pool capacity at some commercial reactors, some cooled spent fuel has
been moved to dry storage casks. The NRC has licensed 30 independent spent fuel storage
installations (ISFSI)for dry casks in 23 states.9 Fuel debris from the 1979 Three Mile Island
reactor accident has been moved to interim storage at the Idaho National Laboratory (INL).
General Electric Company (GE) operates an independent spent fuel storage installation (Morris
Operation) in Morris Illinois. A group of eight electric utility companies has partnered as Private
Fuel Storage, LLC with the Skull Valley Band of Goshute Indians, and applied for an NRC
license to build and operate a temporary facility to store commercial spent nuclear fuel on the
Indian reservation in Skull Valley, Utah.
DOE spent fuel originated from nuclear weapons production, the naval reactor program, and both
domestic and foreign research reactor programs. DOE spent fuel remains in interim storage at
federal sites in Savannah River, South Carolina; Hanford, Washington; INL; and Fort St. Vrain,
Colorado.10
In contrast to commercial reactors, naval reactors can operate without refueling for up to 20
years. 11 As of 2003, 103 naval reactors were in operation, and nearly as many have been
decommissioned from service. Approximately 65 metric tons heavy metal (MTHM) of spent-fuel
have been removed from the naval reactors. Until 1992, naval spent fuel had been reprocessed for
weapons production, and since then has been transferred to INL for interim storage.
The planned Yucca Mountain repository is scheduled to receive 63,000 MTHM commercial spent
nuclear fuel, and 2,333 MTHM of DOE spent-fuel. 12 The NWPA prohibits disposing of more than
the equivalent of 70,000 MTHM in the first repository until a second is constructed.
The Energy Information Administration reported an aggregate total 47,023.4 MTHM discharged
from commercial rectors over the period of 1968 to 2002.13 Of the total, 46,268 MTHM is stored
at reactor sites, and the balance of 755.4 MTHM is in stored away from reactor sites.
8
69 pressurized water reactors (PWR) and 35 boiling water reactors (BWR): U.S. Nuclear Reactors, U.S. DOE, Energy
Information Administration, at http://www.eia.doe.gov/cneaf/nuclear/page/nuc_reactors/reactsum.html.
9
U.S. NRC, 2004-2005 Information Digest, Figure 42—Licensed Operating Independent Spent Fuel Storage
Installations.
10
U.S. DOE Office of Civilian Radioactive Waste Management, Appendix A, Final Environmental Impact Statement
for the Disposal of Spent Nuclear Fuel and High-Level Radioactive Waste at Yucca Mountain, Nye County, Nevada
(DOE/EIS-0250), February 2002.
11
U.S DOE and Department of the Navy, The United States Navy Nuclear Propulsion Program, March 2003.
12
Appendix A—Final Environmental Impact Statement.
13
U.S. DOE Energy Information Administration, Spent Nuclear Fuel Data, Detailed United States as of December 31,
2002, at http://www.eia.doe.gov/cneaf/nuclear/spent_fuel/ussnfdata.html.
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Radioactive Waste Streams: Waste Classification for Disposal
CRS obtained and compiled raw data from EIA on spent fuel discharged by commercial reactor
operators to the end of 2002, and data on spent fuel stored at the DOE national laboratory and
defense sites (as of 2003 year-end).14 A combined total of 49,333 MTHM had been discharged by
commercial- and defense-related activities at the end of 2002. Commercial reactor storage pools
accounted for 41,564 MTHM, and ISFSIs accounted for 5,294 MTHM. The balance was made up
by 2,475 MTHM of federal spent fuel stored at national laboratories, defense sites, and university
research reactors.15 CRS’s figures differ from EIA’s in several respects: EIA compiles only
commercial spent fuel data, combines data on reactor storage pool and dry storage at the reactor
facility site, and identifies non-reactor site spent fuel as “away from reactor site” storage.16 The
data are geographically presented in Figure 2 and summarized in Table 3.
At the end of 1998, EIA reported 38,418 MTHM of spent fuel discharged. 17 Based on 47,023
MTHM discharged at the end of 2002, CRS estimates that commercial reactor facilities discharge
an average 2152 MTHM of spent fuel annually. On that basis, CRS estimates 53,637 MTHM of
spent fuel had been discharged at the end of 2004.
14
15
U.S. DOE Energy Information Administration, Form RW-859, “Nuclear Fuel Data” (2002)
Idaho National Engineering and Environmental Laboratory INTEC Programs Division
16
Mostly General Electric’s Morris facility, and the Fort St. Vrain High Temperature Gas Reactor facility in DOE
caretaker status.
17
U.S. DOE Energy Information Administration, Prior Years 1998 Table, at http://www.eia.doe.gov/cneaf/nuclear/
spent_fuel/ussnfdata.html.
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Figure 2. Federal Sites, Commercial Reactor Storage Pools, and Independent Spent Fuel Storage Installations
Source: U.S. DOE National Laboratories as of 2003 year end, and U.S. DOE EIA Form RW-859 as of 2002 year end.
Note: Numbered labels refer to facilities in Table 3.
CRS-8
Table 3. Federal Site, Commercial Reactor Pool, and Independent Spent Fuel Storage
Facility
St
T
Assembly
MTHM
Facility
St
T
Assembly
MTHM
1. Arkansas Nuclear One
AK
P
1,517
666.7
46. Shearon Harris Nuclear Power Plant
NC
P
3,814
964.5
I
552
241.4
47. Cooper Nuclear Station
NE
P
1,537
278.6
2. Browns Ferry Nuclear Plant
AL
P
6,696
1,230.2
48. Fort Calhoun Nuclear Station
NE
P
839
305.0
3. J M Farley Nuclear Plant
AL
P
2,011
903.8
49. Seabrook Nuclear Station
NH
P
624
287.2
4. Palo Verde Nuclear Generating Station
AZ
P
2,747
1,157.8
50. Hope Creek Generating Station
NJ
P
2,376
431.5
5. Diablo Canyon Power Plant
CA
P
1,736
760.9
2,556
455.9
CA
I
0
0.2
NJ
P
6. GE Vallecitos Nuclear Center
51. Oyster Creek Generating Station
I
244
47.6
7. Humboldt Bay Power Plant
CA
P
390
28.9
52. Salem Nuclear Generating. Station
NJ
P
1,804
832.7
8. Rancho Seco Nuclear Generating Sta
CA
I
493
228.4
53. Sandia National Laboratory
NM
F
503
0.3
9. San Onofre Nuclear Generating Station
CA
P
2,490
1,013.3
54. Brookhaven National Laboratory
NY
F
40
0.0
10. Fort St. Vrain Power Station
CO
F
1,464
14.7
2,460
446.5
CT
P
1,019
412.3
NY
P
11. Connecticut Yankee Atomic Power Co
55. JA Fitzpatrick Nuclear Power Plant
I
204
37.2
12. Millstone Nuclear Power Station
CT
P
4,558
1,227.9
56. Indian Point Energy Center
NY
P
2,073
903.6
13. Crystal River Nuclear Power Plant
FL
P
824
382.3
57. Nine Mile Point Nuclear Station
NY
P
4,456
801.6
14. St. Lucie Nuclear Power Plant
FL
P
2,278
870.7
58. R E Ginna Nuclear Power Plant
NY
P
967
357.4
15. Turkey Point Station
FL
P
1,862
851.7
749
351.3
GA
P
1,639
720.8
OH
P
16. AW Vogtle, Jr. Electric Gen Plant
59. Davis-Besse Nuclear Power Station
I
72
33.9
17. EL Hatch Nuclear Plant
GA
P
5,019
909.3
60. Perry Nuclear Power Plant
OH
P
2,088
378.4
I
816
151.2
61. Trojan Nuclear Power Plant
OR
P
780
358.9
18. D Arnold Energy Center
IA
P
1,912
347.9
62. Beaver Valley Power Station
PA
P
1,456
672.9
19. Idaho National Eng & Env Lab
ID
F
93,705
300.2
63. Limerick Generating Station
PA
P
4,601
824.0
20. Argonne National Lab East
IL
F
78
0.1
5,905
1,062.7
IL
P
1,485
628.7
PA
P
21. Braidwood Generating Station
64. Peach Bottom Atomic Power Sta
I
1,020
190.3
22. Byron Generating Station
IL
P
1,786
756.4
4,240
738.4
IL
P
1,580
288.8
PA
P
23. Clinton Power Station
65. Susquehanna Steam Electric Station
I
1,300
238.5
CRS-9
Facility
St
T
Assembly
MTHM
Facility
St
T
Assembly
MTHM
24. Dresden Generating Station
IL
P
5,698
1,009.2
66. Three Mile Island Nuclear Station
PA
P
898
416.1
I
1,155
146.9
67. Catawba Nuclear Station
SC
P
1,780
782.4
25. General Electric Morris Op
IL
I
3,217
674.3
344
147.9
IL
P
4,106
744.6
SC
P
26. LaSalle County Generating Station
68. HB Robinson Steam Electric Plant
I
56
24.1
27. Quad Cities Generating Station
IL
P
6,116
1,106.5
1,419
665.8
IL
P
2,226
1,019.4
SC
P
28. Zion Generating Station
69. Oconee Nuclear Station
I
1,726
800.4
29. Wolf Creek Generating Station
KS
P
925
427.3
70. Savannah River Defense Site
SC
F
9,657
28.9
30. River Bend Station
LA
P
2,148
383.9
71. VC Summer Nuclear Station
SC
P
812
353.9
31. Waterford Generating Station
LA
P
960
396.4
72. Sequoyah Nuclear Power Plant
TN
P
1,699
782.6
32. Pilgrim Nuclear Station
MA
P
2,274
413.9
73. Watts Bar Nuclear Plant
TN
P
297
136.6
33. Yankee Rowe Nuclear Power Station
MA
I
533
127.1
74. Comanche Peak Steam Electric Station
TX
P
1,273
540.7
34. Calvert Cliffs Nuclear Power Plant
MD
P
1,348
518.0
75. South Texas Project
TX
P
1,254
677.8
I
960
368.1
76. North Anna Power Station
VA
P
1,410
652.7
I
480
220.8
77. Surry Power Station
VA
P
794
365.4
I
1,150
524.2
78. Vermont Yankee Generating Station
VT
P
2,671
488.4
79. Columbia Generating Station
WA
P
1,904
333.7
I
340
61.0
35. Maine Yankee Atomic Power Plant
ME
I
1,434
542.3
36. Big Rock Point Nuclear Plant
MI
I
441
57.9
37. D C Cook Nuclear Plant
MI
P
2,198
969.0
38. Enrico Fermi Atomic Power Plant
MI
P
1,708
304.6
39. Palisades Nuclear Power Station
MI
P
649
260.7
I
432
172.4
40. Monticello Nuclear Generating Plant
MN
P
1,342
236.1
80. Hanford Defense Site
WA
F
110,140
2,128.9
41. Prairie Island Nuclear Gen. Plant
MN
P
1,135
410.3
81. Kewaunee Nuclear Power Plant
WI
P
904
347.6
I
680
262.3
82. La Crosse Nuclear Generating. Station
WI
P
333
38.0
42. Callaway Nuclear Plant
MO
P
1,118
479.0
1,353
507.4
MS
P
3,160
560.2
WI
P
43. Grand Gulf Nuclear Station
83. Point Beach Nuclear Plant
I
360
144.1
44. Brunswick Steam Electric Plant
NC
P
2,227
477.4
45. W B McGuire Nuclear Station
NC
P
2,232
1,001.1
F
4,834
1.7
CRS-10
84. University Research & Domestic Training Reactors
Facility
St
T
Assembly
MTHM
Facility
St
Commercial Reactor Pool
P
145,589
41,564.1
Commercial ISFSI
National Lab & Defense Site Storage
F
220,421
2,474.8
Combined Total
T
Assembly
MTHM
I
18,630
5,294.6
384,640
49,333.4
Totals by Type (T):
CRS-11
Radioactive Waste Streams: Waste Classification for Disposal
High-Level Radioactive Waste
NWPA defines high-level waste as “liquid waste produced directly in reprocessing and any solid
material derived from such liquid waste that contains fission products in sufficient
concentrations,” and “other highly radioactive material” that NRC determines requires permanent
isolation.18 Most of the United States’ high-level waste inventory was generated by DOE (and
former AEC) nuclear weapons programs at the Hanford, INL, and Savannah River Sites. A
limited quantity of high-level waste was generated by commercial spent fuel reprocessing at the
West Valley Demonstration Project in New York.19 Over concern that reprocessing contributed to
the proliferation of nuclear weapons, President Carter terminated federal support for commercial
reprocessing in 1977. For further information on reprocessing policy, refer to CRS Report
RS22542, Nuclear Fuel Reprocessing: U.S. Policy Development, by (name redacted).
Weapons-production reactor fuel, and naval reactor spent fuel were processed to remove special
nuclear material (plutonium and enriched uranium). Reprocessing generated highly radioactive,
acidic liquid wastes that generated heat.20 Weapons-related spent fuel reprocessing stopped in
1992, ending high-level waste generation in the United States. The wastes that were previously
generated continue to be stored at Hanford, INL, and Savannah River, where they will eventually
be processed into a more stable form for disposal in a deep geologic repository.
The Hanford Site generated approximately 53 million gallons of high-level radioactive and
chemical waste now stored in 177 underground carbon-steel tanks. 21 Some strontium and cesium
had been separated out and encapsulated as radioactive source material, then commercially leased
for various uses. The Savannah River Site generated about 36 million gallons of high-level waste
that it stored in 53 underground carbon-steel tanks.22 Both the Hanford and Savannah River Sites
had to neutralize the liquid’s acidity with caustic soda or sodium nitrate to condition it for storage
in the carbon-steel tanks. (The neutralization reaction formed a precipitate which collected as a
sludge on the tank bottom; see the discussion of waste-incidental-to-reprocessing below.)
Savannah River has constructed and begun operating a defense-waste processing facility that
converts high-level waste to a vitrified (glass) waste-form. The vitrified waste is poured into
canisters and stored on site until eventual disposal in a deep geologic repository. A salt-stone
18
“Permanent isolation” is left undefined by the NWPA.
From 1966 to 1972, Nuclear Fuel Services operated a commercial nuclear fuel reprocessing plant at the Western
New York Nuclear Services Center under contract to the State of New York. During the six years of operation, the
plant processed approximately 640 metric tons of spent nuclear fuel, about three-fourths of which was provided by the
AEC (60 percent of the total was from U. S. defense reactors). The plant generated approximately 2.3 million liters
(600,000 gallons) of liquid high-level waste that was stored in underground tanks. In 1972, nuclear fuel reprocessing
operations were discontinued. The liquid high-level radioactive waste produced during reprocessing was stored in
underground steel tanks. New York State Energy Research and Development Authority, at http://www.nyserda.org/
westval.html.
20
U.S. DOE, Integrated Data Base Report—1995: U.S. Spent Nuclear Fuel and Radioactive Waste Inventories,
Projections, and Characteristics, Rev. 12 (DOE/RW-0006), December 1996.
21
U.S. DOE Hanford Site, Electricity, Water, and Roads for Hanford’s Future Vitrification Plant Completed Ahead of
Schedule and Under Budget, press release, September 18, 2001, at http://www.hanford.gov/press/2001/orp/orp091801.html.
22
U.S. DOE Savannah River Site, Spent Nuclear Fuel Program Fact Sheet, at http://www.srs.gov/general/outreach/srscab/fuelfrm/facts1.htm.
19
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byproduct will be permanently disposed of on site. Hanford has plans for a similar processing
facility.
INL generated approximately 300,000 gallons of high-level waste through 1992 by reprocessing
naval reactor spent fuel, and sodium-bearing waste from cleaning contaminated facilities and
equipment. 23 The liquid waste had originally been stored in 11 stainless steel underground tanks.
All of the liquid high-level waste has been removed from five of the 11 tanks and thermally
converted to granular (calcine) solids. Further treatment is planned, and INL is also planning a
waste processing facility similar to Savannah River’s vitrification plant.
West Valley’s high-level waste has been vitrified and removed from the site. The vitrification
process thermally converts waste materials into a borosilicate glass-like substance that chemically
bonds the radionuclides. The vitrification plant is being decommissioned. The Hanford Site and
INL are planning similar vitrification plants.
High-level waste is also considered a mixed waste because of the chemically hazardous
substances it contains, which makes it subject to the environmental regulations under the
Resource Conservation and Recovery Act (RCRA).
Waste Incidental to Reprocessing
DOE policy in Order 435.1 refers to waste incidental to reprocessing in reclassifying a waste
stream that would otherwise be considered high-level due to its source or concentration.24 DOE’s
Implementation Guide to the Order states that “DOE Manual 435.1-1 is not intended to create, or
support the creation of, a new waste type entitled incidental waste.” The waste stream typically
results from reprocessing spent fuel. DOE has determined that under its regulatory authority the
incidental-to-processing waste stream can be managed according to DOE requirements for
transuranic or low-level waste, if specific criteria are met.
The DOE evaluation process for managing spent-fuel reprocessing wastes considers whether (1)
the “wastes are the result of reprocessing plant operations such as contaminated job wastes
including laboratory items such as clothing, tools and equipment,”25 and (2) key radionuclides
have been removed in order to permit downgrading the classification to either low-level waste or
transuranic waste. Evaluation process wastes include large volumes of low-activity liquid wastes
(separated from high-level waste streams), a grout or salt-stone solid form, and high-level waste
residues remaining in storage tanks. DOE’s evaluation process at the Savannah River Site resulted
in capping the residue left in high-level waste storage tanks with cement grout.
Public comments on the draft of Order 435.1 expressed the concern that potentially applicable
laws do not define or recognize the principle of “incidental waste,” or exempt high-level waste
that is “incidental” to DOE waste management activities from potential NRC licensing
23
U.S. DOE Idaho National Laboratory/ Idaho Nuclear Technology and Engineering Center—Cleanup Status, at
http://www.inel.gov/ environment/intec/.
24
U.S. DOE, M 435.1-1 Radioactive Waste Management Manual of 7-09-99, and G 435.1-1 Implementation Guide for
DOE M 435.1-1.
25
Notice of Proposed Rulemaking (34 FR 8712) for Appendix D 10 C.F.R. 50.
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authority. 26 In 2003, the Natural Resources Defense Council (NRDC) challenged DOE’s
evaluation process for Savannah River as scientifically indefensible, since no mixing occurred to
dilute the residue’s activity when capping it with grout.27 DOE countered that through the wasteincidental-to-reprocessing requirements of Order 435.1, key radionuclides have been removed
from the tanks, and the stabilized residual waste does not exceed Class C low-level radioactive
waste restrictions for shallow land burial.28 Removing the residual waste would be costly and
expose workers to radiologic risks, according to DOE.
In NRDC v. Abraham, the Federal District Court in Idaho ruled in 2003 that DOE violated the
NWPA by managing wastes through the evaluation process in Order 435.1.29 The Energy
Secretary later asked the Congress for legislation clarifying DOE authority in determinations on
waste-incidental-to-reprocessing at Hanford, Savannah River, and INL.30 On November 5, 2004,
the U.S. Court of Appeals for the Ninth Circuit vacated the district court’s judgment and
remanded the case with a direction to dismiss the action.31
Section 3116 (Defense Site Acceleration Completion) in the Ronald W. Reagan Defense
Authorization Act of FY2005 (P.L. 108-375) specified that the definition of the term “high-level
radioactive waste” excludes radioactive waste from reprocessed spent fuel if (1) the Energy
Secretary in consultation with the NRC determines the waste has had highly radioactive
radionuclides removed to the maximum extent practical, and (2) the waste does not exceed
concentration limits for Class C low-level waste. As a result of the Act, NRC expects to review an
increased number of waste determinations. As guidance to its staff, NRC developed a draft
Standard Review Plan (NUREG-1854). 32 Section 3117 of the Act (Treatment of Waste Material)
authorizes $350 million for DOE’s High Level Waste Proposal to accelerate the cleanup schedule
for the Hanford, Savannah River, and INL. For further information on this subject, refer to CRS
Report RS21988, Radioactive Tank Waste from the Past Production of Nuclear Weapons:
Background and Issues for Congress, by (name redacted) and (name redacted).
Transuranic Waste
The Atomic Energy Act (42 U.S.C. 2014) defines transuranic (TRU) waste as material
contaminated with elements having atomic numbers greater than uranium (92 protons) in
concentrations greater than 10 nanocuries/gram. The DOE (with other federal agencies) revised
the minimum radioactivity defining transuranic waste from 10 nanocuries/gram to greater than
100 nanocuries/gram in 1984.
26
U.S. DOE Office of Environmental Management, Summary of Public Comments on DOE Order 435.1, Radioactive
Waste Management, at http://web.em.doe.gov/em30/pubsum16.html.
27
Letter from Natural Resources Defense Council to the Honorable J. Dennis Hastert, August 19, 2003.
28
Second Declaration of Jessie Roberson in NRDC v. Abraham, 271 F. Supp. 2nd 1260 (D. Id. 2003).
29
NRDC v. Abraham, 271 F. Supp. 2nd 1260 (D. Id. 2003).
30
“DOE seeks nuclear waste clarification to reaffirm HLW disposal strategy,” Nuclear Fuel, The McGraw-Hill
Companies, August 19, 2003.
31
No. 03-35711 United States Court of Appeals for the Ninth Circuit 2004 U.S.
32
U.S. NRC, Standard Review Plan for Activities Related to U.S. Department of Energy Waste Determinations—Draft
Report For Interim Use and Comment (NUREG-1854), May 2006.
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Transuranic elements are artificially created in a reactor by irradiating uranium. These elements
include neptunium, plutonium, americium, and curium. Many emit alpha particles and have long
half-lives. 33 Americium has commercial use in smoke detectors, and plutonium produces fission
energy in commercial power reactors.
Transuranic waste is generated almost entirely by DOE (and former AEC) defense-related
weapons programs. The waste stream results from reprocessing irradiated fuel to remove
plutonium-239 or other transuranic elements, and from fabricating nuclear weapons and
plutonium-bearing reactor fuel. The waste may consist of plutonium-contaminated debris (such as
worker clothing, tools, and equipment), sludge or liquid from reprocessing, or cuttings and scraps
from machining plutonium.
In 1970, the former AEC determined that the long half-life and alpha emissions associated with
transuranic waste posed special disposal problems. This prompted the decision to stop the
practice of burying TRU waste in shallow landfills as a low-level waste.34
DOE distinguishes “retrievably stored” transuranic waste from “newly generated” waste. Waste
buried prior to 1970 is considered irretrievable and will remain buried in place. Since 1970,
transuranic waste has been packaged (e.g., metal drums, wood or metal boxes) and retrievably
stored in above-ground facilities such as earth-mounded berms, concrete culverts, buildings, and
outdoor storage pads. Waste that has been retrieved or will be retrieved, and then repackaged for
transportation and disposal, is classed as newly generated waste.35
The Department of Energy National Security and Military Applications of Nuclear Energy
Authorization Act of 1980 (P.L. 96-164) directed the Energy Secretary to consult and cooperate
with New Mexico in demonstrating the safe disposal of defense radioactive wastes. The Waste
Isolation Pilot Plant Land Withdrawal Act (P.L. 102-579 as amended by P.L. 104-211) limited
disposal acceptance to transuranic waste with a half-life greater than 20 years and radioactivity
greater than 100 nanocuries/gram. The WIPP Act further defined transuranic waste in terms of
“contact-handled transuranic waste” having a surface dose less than 200 millirem per hour, and
“remote-handled transuranic waste” having a surface dose rate greater than 200 millirem/hour.
The WIPP facility (near Carlsbad, New Mexico) began accepting transuranic waste in 1999 but
was restricted by the New Mexico Environment Department to accepting contact-handled waste
only. In October 2006, New Mexico revised WIPP’s permit to allow remote-handled waste.
The Resource Conservation and Recovery Act of 1976 (42 U.S.C. 6901) imposed additional
disposal requirements on transuranic waste mixed with hazardous constituents. Mixed radioactive
and hazardous waste is a separate classification discussed further below.
The Energy and Water Development Appropriations Act for 2005 (P.L. 108-447) and
appropriation acts for some prior years precluded the WIPP facility from disposing of transuranic
waste containing plutonium in excess of 20%, as determined by weight.
33
Arjun Makhijani and Scott Saleska, High-level Dollars, Low-Level Sense, The Apex Press, New York, 1992.
U.S. DOE, Integrated Data Base Report-1995: U.S. Spent Nuclear Fuel and Radioactive Waste Inventories,
Projections, and Characteristics (DOE/RW-0006, Rev.12), December, 1996.
35
The National Academies Board on Radioactive Waste Management, Characterization of Remote-Handled
Transuranic Waste for the Waste Isolation Pilot Plant, Interim Report, National Academy Press, Washington, D.C.,
2001.
34
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Radioactive Waste Streams: Waste Classification for Disposal
Surplus Weapons-Usable Plutonium
The Atomic Energy defined “special nuclear material” as plutonium, uranium enriched in
isotopes 233 or 235, and any other material the NRC determined as special nuclear material.
Special nuclear material is important in weapons programs and as such has strict licensing and
handling controls. Under President Clinton’s 1993 Nonproliferation and Export Control Policy,
55 tons of weapons-usable plutonium was declared surplus to national security needs.36 DOE
plans to use surplus plutonium in mixed oxide fuel for commercial power reactors.37 Plutonium
not suitable for mixed oxide fuel fabrication is destined for repository disposal. The special
facility constructed to reprocess the surplus would generate transuranic waste and low-level
radioactive waste streams. Spent mixed oxide fuel would be disposed of in the same manner as
conventional commercial spent fuel in an NRC-licensed deep geologic repository.
Low-Level Radioactive Waste
The Low-Level Radioactive Waste Policy of 1980 (P.L. 96-573) defined “low-level radioactive
waste” as radioactive material that is not high-level radioactive waste, spent nuclear fuel, or
byproduct material, and radioactive material that the Nuclear Regulatory Commission (NRC)
classifies as low-level radioactive waste consistent with existing law. Low-level waste is
classified as A, B, C, or Greater than Class C in 10 C.F.R. 61.55—Waste Classification. These
classes are described further below. Commercial low-level waste is disposed of in facilities
licensed under NRC regulation, or NRC-compatible regulations of “agreement states.”
Low-level radioactive waste is generated by nuclear power plants, manufacturing and other
industries, medical institutions, universities, and government activities. Much of the nuclear
power plant waste comes from processes that control radio-contaminants in reactor cooling water.
These processes produce wet wastes such as filter sludge, ion-exchange resins, evaporator
bottoms, and dry wastes. Institutions such as hospitals, medical schools, research facilities, and
universities generate wastes of significantly differing characteristics. Industrial generators
produce and distribute radionuclides, and use radioisotopes for instruments and manufacturing
processes. The General Accounting Office (now Government Accountability Office) reported that
of the 12 million cubic feet of low-level waste disposed of in 2003, 99% constituted Class A. 38
The NRC classifies low-level waste using two tables: one for long-lived radionuclides, and one
for short-lived. Long-lived and short-lived refer to the length of time for radioactive decay. For
regulatory purposes, the dividing line between short-lived and long-lived is a half-life of 100
years. The radionuclides included as long-lived are: carbon-14, nickel-59, niobium-94,
technetium-99, iodine-129, plutonium-241, and curium-242. The group “alpha emitting
transuranic nuclides with half-lives greater than 5 years” is included in the long-lived table, as
various isotopes of the group may have half-lives in the range of hundreds-of-thousand of years.
36
U.S. DOE Office of Fissile Materials Disposition, Surplus Plutonium Disposition Final Environmental Impact
Statement (TIC:246358), 1999.
37
U.S. DOE, Record of Decision for the Surplus Plutonium Final Environmental Impact Statement, 65 FR 1608;
January 11, 2000.
38
U.S. GAO, Low-Level Radioactive Waste—Disposal Availability Adequate in the Short Term, but Oversight Needed
to Identify Any Future Shortfalls (GAO-04-604), June 2004.
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Radioactive Waste Streams: Waste Classification for Disposal
The short-lived radionuclide table includes tritium (hydrogen-3), cobalt-60, nickel-63, strontium90, and cesium-137. A group of unspecified “nuclides with half-lives less than 5 years” is
included as short-lived.
Low-level waste generated by nuclear power plants results from the fission of uranium fuel, or
the activation of the reactor components from neutrons released during fission. Trace amounts of
uranium left on fuel rod surfaces during manufacturing are partly responsible for the fission
products in the reactor cooling water.39 Tritium (H-3) occasionally results from uranium fission,
and from reactor cooling water using boron as a soluble control absorber.40 The radionuclides
carbon-14, nickel-53, nickel-59, and niobium-94 are created when stainless steel reactor
components absorb neutrons. The radionuclides strontium-90, technetium-99, and cesium-137 are
fission products of irradiated uranium fuel. The transuranic radionuclides are neutron-activation
products of irradiated uranium fuel. Iodine-129 is found in radioactive wastes from defenserelated government facilities and nuclear fuel cycle facilities; if released into the environment, its
water solubility allows its uptake by humans, where it concentrates in the thyroid gland.41
Some of the short-lived radionuclides have specific industrial or institutional applications. These
include cobalt-60, strontium-90, and cesium-137. Cobalt-60 is used in sealed sources for cancer
radiotherapy and sterilization of medical products; its intense emission of high-energy gamma
radiation makes it an external hazard, as well as an internal hazard when ingested. Strontium-90
is used in sealed sources for cancer radiotherapy, in luminous signs, in nuclear batteries, and in
industrial gauging. Due to strontium’s chemical similarity to calcium, it can readily be taken up
by plants and animals, and is introduced into the human food supply through milk. Cesium-137
also is used in sealed sources for cancer radiotherapy, and due to its similarity to potassium can be
taken up by living organisms.
Low-level waste classification ultimately determines whether waste is acceptable for shallow land
burial in an NRC- or state-licensed facility. The four waste classes identified by 10 C.F.R. Section
61.55 on the basis of radionuclide concentration limits are:
•
Class A: waste containing the lowest concentration of short-lived and long-lived
radionuclides. Examples include personal protective clothing, instruments, tools,
and some medical wastes. Also, waste containing any other radionuclides left
unspecified by 10 C.F.R. 61.55 is classified as A.
•
Class B: an intermediate waste classification that primarily applies to waste
containing either short-lived radionuclides exclusively, or a mixture of shortlived and long-lived radionuclides in which the long-lived concentration is less
than 10% of the Class C concentration limit for long-lived radionuclides.
•
Class C: wastes containing long-lived or short-lived radionuclides (or mixtures of
both) at the highest concentration limit suitable for shallow land burial. Examples
include ion exchange resins and filter materials used to treat reactor cooling
water, and activated metals (metal exposed to a neutron flux—irradiation—that
creates a radioactive isotope from the original metal).
39
U.S. DOE, Appendix A, Final Environmental Impact Statement.
Raymond, L. Murray, Chapter 16 of Understanding Radioactive Waste, Battelle Press, 2003.
41
U.S. EPA, Facts about Iodine, at http://www.epa.gov/superfund/resources/radiation/pdf/iodine.pdf.
40
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Radioactive Waste Streams: Waste Classification for Disposal
•
Greater than Class C (GTCC): waste generally not acceptable for near-surface
disposal. Greater than Class C wastes from nuclear power plants include
irradiated metal components from reactors such as core shrouds, support plates,
and core barrels, as well as filters and resins from reactor operations and
decommissioning.
The physical form, characteristics, and waste stability requirements are summarized in Table 4.
Table 4. Physical Form and Characteristics of Low-Level Waste
Greater than
Class C
Class A
Class B
Class C
Form
Trash, soil, rubble,
depleted uranium,
mildly contaminated
equipment and
clothing.
Reactor components,
sealed radioactive
sources, filters and
resins from nuclear
power plants.
Same as Class B but
higher in radioactivity.
Reactor components
and filter resins from
reactor
decommissioning.
Specific activity
near background to
700 Ci/m3
0.04 to 700 Ci/m3
44 to 7,000 Ci/m3
Greater than Class C.
Maximum
waste
concentration
basis
•
•
•
100-year decay
exceeds
acceptable
hazard levela to
an intruder.
Unspecified by
regulation.
•
500-year
acceptable
hazard level
reached.
•
500-year
protection
provided by
deeper disposal
or intruder
barriers.
100-year decay
to acceptable
hazard level* to
an intruder
100-year decay
to acceptable
hazard level* to
an intruder.
Waste
containers
No special provisions,
if waste is buried in a
separate disposal cell.
Must be designed to
be stable for 300
years.
Must remain stable
for 300 years.
(Not applicable)
Special
Disposal
Provisions
Waste stabilization
required if buried
with Class B or C
waste.
(Not applicable)
Barriers to intrusion
required that must
remain effective for
500 years where site
conditions prevent
deeper disposal.
Though generally not
acceptable for nearsurface disposal,
regulation allows for
disposal in nearsurface facility if
approved by NRC, or
other wise must be
disposed of in a
geologic repository.
Note: Ci/m3: Curies/cubic-meter
a.
Acceptable hazard level to an intruder is based on maximum annual dose equivalent of 500 millirem (mrem)
to the whole body of any member of the public—Sec. 61.42, and draft Generic Environmental Impact
Statement for Part 61, NUREG-0782. Acceptable hazard level to the general population is based on
maximum dose equivalent of 25 mrem to whole body, 75 millirems to thyroid, and 25 millirems to any
organ of any member of the public.
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Class A, B, and C wastes are candidates for near-surface disposal. The concept for near-surface
disposal is: a system composed of the waste form, a trenched excavation, engineered barriers, and
natural site characteristics. Through complex computer models, the licensee must demonstrate
that the site and engineered features comply with the performance objectives in 10 C.F.R. Part 61.
Generally Class A and B wastes are buried no greater than 30 meters (~100 feet). Class C waste
must be buried at a greater depth to prevent an intruder from disturbing the waste after
institutional controls have lapsed. The operation of a disposal facility was originally foreseen to
last 20 to 40 years, after which it would be closed for stabilization period of 1 to 2 years,
observed and maintained for 5 to 15 years, then transferred to active institutional control for 100
years.42 At the time of licensing, funds had to be guaranteed by the state or licensee for the
facility’s long term care after closure. At present, no disposal facility exists for Greater than Class
C Waste, though the DOE is in the initial phase of a process to identify disposal options.43
The Senate Committee on Energy and Natural Resources conducted a hearing in September 2004
to consider the potential shortage of low-level waste disposal sites.44 The GAO had concluded in
a 2004 report that no shortfall in disposal capacity appeared imminent, although the national lowlevel waste database that would be used to estimate the adequacy of future capacity was
inaccurate.45 The GAO recommended that the DOE stop reporting the database information, and
added that Congress may wish to consider directing the Nuclear Regulatory Commission to report
when the disposal capacity situation changes enough to warrant congressional evaluation.
Provisions for State Disposal Compacts
In enacting the Low-Level Radioactive Waste Policy Act of 1980, Congress also established the
policy that each state take responsibility for disposing of low-level radioactive waste generated
within its borders. To accomplish this, states may enter into compacts. Section 102 of the 1986
amendments to the Act provided that each state, either by itself or in cooperation with other
states, be responsible for disposing of low-level radioactive wastes generated within the state.
Low-Level Waste Classification Tables
The NRC created two tables in 10 C.F.R 61.55 for classifying low-level waste on the basis of
radionuclide concentration limits. Table 1 of the regulation applies to long-lived radionuclides,
and Table 2 applies to short-lived (included as Figures A-1 and A-2 in the Appendix of this
report). The concentration limits are expressed in units of “curies/cubic meter” or
“nanocuries/gram” (the latter unit applying exclusively to the alpha-emitting transuranic
radionuclides). Figures 3 through 6 represent an illustrative guide to interpreting Tables 1 and 2;
they are not intended, however, for actual waste classification purposes. The figures break down
Tables 1 and 2 by long-lived, transuranic, short-lived and mixed long- and short-lived
radionuclides. In the case of mixed radionuclides, the “sum-of-the-fractions” rule must be
applied.
42
U.S. NRC, Final Environmental Impact Statement on 10 CFR Part 61 “Licensing Requirements for Land Disposal of
Radioactive Waste (NURGEG-0945), November 1982.
43
“DOE begins looking at options for disposal of GTCC radwaste,” Nuclear Fuels, October 11, 2004.
44
S. Hrg. 108-756, September 30, 2004.
45
U.S. GAO, Low-Level Radioactive Waste—Disposal Availability Adequate in the Short Term, but Oversight Needed
to Identify Any Future Shortfalls (GAO-04-604), June 2004.
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Radioactive Waste Streams: Waste Classification for Disposal
Sum-of-the-Fractions Rule. Waste containing a mixture of radionuclides must be classified by
applying the sum-of-the fractions rule. In the case of short-lived radionuclides—for each
radionuclide in the mixture, calculate the fraction:
radionuclide-concentration
lowest-concentration-limit
then calculate the fractions’ sum. If the sum-of-the-fractions is less than 1, the waste class is Class
A. If the sum of the fractions is greater than 1, recompute each fraction using the upper
concentration limits. If the fraction sum is less than 1, the waste is Class C; if greater than 1 then
it is Greater than Class C. In the case of long-lived radionuclides, sum the fractions of each
radionuclide concentration divided by the Column 1 concentration limits. If the resulting fraction
sum is less than 1, the waste is Class A. If the fraction sum is greater than 1, recompute the
fractions by applying the Column 2 concentration limits. If the sum is less than 1, the waste is
Class B. If the sum is greater than 1, recompute again using the Column 3 limits. For example,
consider a waste containing concentrations of long-lived radionuclides Sr-90 at 50 Ci/m3 and Cs137 at 22 Ci/m3. Since the concentrations each exceed the values in Column 1 (0.04 and 1.0
respectively) of Chart 3 (Table 2 of Section 61.55), they must be compared to the concentration
limits of Column 2. For Sr-90, the fraction 50/150 equals 0.33, for Cs-137 the fraction 22/44
equals 0.5. The resulting sum of the fractions (0.33 + 0.5) equals 0.83. Since the sum is less than
1.0, the waste is Class B.
Figure 3. Low-Level Waste Classification by Long-Lived Radionuclides
Source: Congressional Research Service
Notes: Waste Containing Only Long-lived Radionuclides – For waste containing on long-lived radionuclides,
classification is based on the concentration limits in 10 C.F.R. 61.55—Table 1. The concentration limits are
expressed in curies per cubic meter. Note that Class A’s concentration limit is one-tenth of Class C’s limit. Also,
note that Class B is left undefined by §61.55 in the case of waste containing exclusively long-lived radionuclides.
Waste containing mixtures of Table 1 radionuclides must be classified by applying the sum-of-the-fractions rule.
[ ] – indicates activated metal (exposure to a neutron flux resulting in a radioactive isotope of the original
metal).
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Radioactive Waste Streams: Waste Classification for Disposal
Figure 4. Low-Level Waste Classification by Transuranic Radionuclides
Source: Congressional Research Service
Notes: Waste Containing Only Transuranic Radionuclides – For waste containing only transuranic radionuclides
classification is based on the concentration limits of 10 C.F.R. 61.55—Table 1. The concentration limits are
expressed in terms of noncuries per gram. The limit for Class A is one-tenth that for Class C concentrations. As
in the case of long-lived radionuclides, §61.55 leaves Class B undefined for waste containing exclusively
transuranic radionuclides. Waste containing mixtures of Table 1 radionuclides must be classified by applying the
sum-of-the-fractions rule.
ηCurie: 10-9 Curie.
α : alpha particle-emitting transuranic nuclides.
Pu241 decays to Am241 half-life = 460 years, Cm242 decays to Pu238 half-life = 86 years.
Figure 5. Low-Level Waste Classification by Short-Lived Radionuclides
Source: Congressional Research Service
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Radioactive Waste Streams: Waste Classification for Disposal
Notes: Waste Containing Only Short-lived Radionuclides – For waste containing only short-lived radionuclides,
classification is based on the concentration limits in 10 C.F.R. 61.55 Table 2. The concentration limits are
expressed in terms of curies per cubic meter. Note that the concentration limits in Columns 2 and 3 are not
specified for the sum of radionuclides in concentrations above those in Column 1 will be classified as B (unless
other radionuclide concentrations determine the waste to be Class C). The external radiation and internal heat
generated by these radionuclides must be given practical consideration during transportation and handling, and
thus may limit their concentrations. Waste containing mixtures of Table 2 radionuclides must be classified by
applying the sum-of-the-fractions rule.
*No Limit: Practical considerations such as effects of external radiation and internal heat generation on
transportation, handling and disposal will limit the concentrations.
∑t1/2<5y: nuclides with radioactive half-lives less than 5 years.
Figure 6. Low-Level Waste Classification by Mixed Long-Lived and Short-Lived
Radionuclides
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Source: Congressional Research Service
Notes: Waste Containing Mixed Long-lived and Short-lived Radionuclides – Based on the concentration limits of
10 C.F.R. 61.55 – Tables 1 & 2, when long-lived radionuclide concentrations are less than the lower limits, the
waste classification is determined by short-lived concentration limits. If long-lived radionuclide concentrations are
between the lower and upper limits, the waste is classified as C, and above the upper limits as Greater-than
Class C.
*No Limit: Practical considerations such as effects of external radiation and internal heat generation on
transportation, handling and disposal will limit the concentrations.
Mixed Low-Level Radioactive and Hazardous Waste
Mixed waste contains both concentrations of radioactive materials that satisfy the definition of
low-level radioactive waste in the Low-Level Radioactive Waste Policy Act, and hazardous
chemicals regulated under the Resource Conservation and Recovery Act (RCRA, 42 U.S.C.
6901). In general, facilities that manage mixed waste are subject to RCRA Subtitle C (Hazardous
Waste) requirements for hazardous waste implemented by EPA (40 C.F.R. 124 and 260-270) or to
comparable regulations implemented by states or territories that are authorized to implement
RCRA mixed waste authority. The RCRA Subtitle C program was primarily developed for the
states’ implementation with oversight by EPA.
Depleted Uranium
Naturally occurring source material uranium contains uranium isotopes in the approximate
proportions of: U-238 (99.3%), U-235 (0.7%), and U-234 (trace amount) by weight. Source
material uranium is radioactive, U-235 contributing 2.2% of the activity, U-238 48.6%, and U234 49.2% .46 Depleted uranium is defined in 10 CFR 40.4 (Domestic Licensing of Source
Material) as “the source material uranium in which the isotope U-235 is less than 0.711 % of the
total uranium present.” It is a mixture of isotopes U-234, U-235, and U-238 having an activity
less than that of natural uranium.47 Most of the DOE depleted uranium hexafluoride inventory has
between 0.2% and 0.4% U-235 by weight. 48
The former AEC began operating uranium enrichment plants in 1945 to produce U-235 enriched
fuel for national defense and civilian nuclear reactors. Most commercial light-water reactors use
uranium enriched 2%-5% with U-235.49 As part of that enrichment process, uranium ore was
converted to uranium hexafluoride (UF6) gas to facilitate U-235’s separation, depleting the
source material uranium of its U-235 isotope. DOE’s inventory of depleted uranium hexafluoride
(DUF6) is approximately 700,000 metric tons. The DUF6 is stored in metal cylinders at the three
enrichment plant sites: Paducah, KY; Portsmouth, OH; and Oak Ridge, TN.
46
47
U.S. NRC, Natural Uranium, at http://www.nrc.gov/reading-rm/basic-ref/glossary/natural-uranium.html.
ANSI N7.2-1963 definition.
48
U.S. DOE, Office of Environmental Management Depleted Uranium Hexafluoride Management Program, Overview
of Depleted Uranium Hexafluoride Management Program, at http://web.ead.anl.gov/uranium/pdf/
DUF6MgmtOverviewFS.PDF.
49
U.S. DOE National Nuclear Security Administration, Nuclear Terms Handbook, 2001.
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As part of DOE’s DUF6 Management Program, 50 Oak Ridge National Laboratory (ORNL)
conducted an assessment of converting the DUF6 to one of four stable forms: metallic (DU),
tetrafluoride (DUF4), dioxide (DUO2) and triuranium octaoxide (DU3O8).51 ORNL considers the
characteristics of the four forms suitable for disposal as low-level radioactive waste. The DU
metal form has commercial and military uses (aircraft counterweights, shielding, armor, and
munitions).
DOE has considered the environmental impacts, benefits, costs, and institutional and
programmatic needs associated with managing its DUF6 inventory. In the 1999 Record of
Decision for Long Term Management and Use of Depleted Uranium Hexafluoride,52 DOE
decided to convert the DUF6 to depleted uranium oxide, depleted uranium metal, or a
combination of both. The depleted uranium oxide would be stored for potential future uses or
disposal as necessary. Conversion to depleted uranium metal would be performed only when uses
for the converted material were identified. DOE stated that it did not believe that long-term
storage as depleted uranium metal and disposal as depleted uranium metal were reasonable
alternatives. DOE has selected Uranium Disposition Services to design, build and operate
facilities in Paducah and Portsmouth to convert the DUF6. DOE has effectively declared DUF6 a
resource in the record of decision, anticipating its conversion to non-reactive depleted uranium
oxide. Making the material nonreactive is intended to eliminate the RCRA criteria that otherwise
would place it in a Mixed Waste class.
Technologically Enhanced Naturally Occurring
Radioactive Material
Technologically Enhanced Naturally Occurring Radioactive Material (TENORM) is a byproduct
of processing mineral ores containing naturally occurring radionuclides. These include uranium,
phosphate, aluminum, copper, gold, silver, titanium, zircon and rare earth ores. 53 The ore
beneficiation process concentrates the radionuclides above their naturally occurring
concentrations. Some TENORM may be found in certain consumer products, as well as fly ash
from coal-fired power plants. Activities such as treating drinking water also produce TENORM.
Surface and groundwater reservoirs may contain small amounts of naturally occurring
radionuclides (uranium, radium, thorium, and potassium; i.e., NORM). In areas where
concentrations of radium are high in underlying bedrock, groundwater typically has relatively
high radium content. Water treatment/filtration plants may remove and concentrate NORM in a
plant’s filters, tanks, and pipes. The result is technologically concentrated NORM (thus
TENORM) in the form of filtrate and tank/pipe scale. Radium-226, a decay product of uranium
and thorium soluble in water, is a particular concern because of the radiologic threat it poses.
Public exposure to TENORM is subject to federal regulatory control.
At Congress’s request in 1997, the EPA arranged for the National Academy of Sciences (NAS) to
study the basis for EPA’s regulatory guidance on naturally occurring radioactive material. The
50
U.S. DOE, Depleted UF6 Management, at http://web.ead.anl.gov/uranium/mgmtuses/index.cfm.
Oak Ridge National Laboratory, Assessment of Preferred Depleted Uranium Disposal Forms (ORNL/TM-2006/161)
June 2000.
52
U.S. DOE, DUF6 Programmatic EIS, at http://web.ead.anl.gov/uranium/documents/nepacomp/index.cfm.
53
U.S. EPA, TENORM Sources, at http://www.epa.gov/radiation/tenorm/sources.htm#mining_ resources.
51
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NAS study defined technologically enhanced radioactive material (TENORM) as “any naturally
occurring material not subject to regulation under the Atomic Energy Act whose radionuclide
concentrations or potential for human exposure have been increased above levels encountered in
the natural state by human activities.” The NAS completed its study in 1999.54 The most
important radionuclides identified by the study include the long-lived naturally occurring isotopes
of radium, thorium, uranium, and their radiologically important decay products. Radium is of
particular concern because it decays to form radioactive radon gas, a carcinogen contributing to
lung cancer. NAS noted that federal regulation of TENORM is fragmentary. Neither the EPA nor
any other federal agency with responsibility for regulating radiation exposure has developed
standards applicable to all exposure situations that involve naturally occurring radioactive
material.
The EPA submitted its own report on implementing the NAS recommendations to Congress the
following year, along with plans to revise its TENORM guidance documents.55 According to its
website, the EPA has used its authority under a number of existing environmental laws to regulate
some sources of TENORM, including the Clean Air Act, the Clean Water Act, the Safe Drinking
Water Act, and the Comprehensive Environmental Response, Compensation, and Liability Act
(CERCLA).56
Energy Policy Act Provisions for NORM
The Energy Policy Act of 200557 contains a provision in Section 651 that amends the Atomic
Energy Act’s section 11(e) definition of “byproduct material” to exclude “any discrete source of
naturally occurring radioactive material [NORM], other than source material” that the NRC, in
consultation with the EPA, Department of Energy, and Department of Homeland Security,
determines would pose a threat similar to the threat posed by a discrete source of radium-226.
The Energy Policy Act also made clear that byproduct material as defined in paragraphs (3) and
(4) of section 11(e) is not to be considered low-level radioactive waste for the purpose of disposal
under the Low-Level Radioactive Waste Policy Act and “carrying out a compact” under the
authorization of 42 U.S.C. sections 2021(b) et seq. 58 (permitting NRC agreements with states to
discontinue its regulatory authority over byproduct, source, and special nuclear materials.)
The Nuclear Regulatory Commission (NRC) proposes to amend its regulations to include
jurisdiction over certain radium sources, accelerator-produced radioactive materials (referred to as
NARM).59 The proposed rule does not suggest any discrete source of NARM nor criteria for
making such a determination. It does note that EPAct gives the NRC authority over discrete
sources of radium-226 but not over diffuse sources of radium-226 as it occurs in nature or over
54
National Research Council Committee on Evaluation of EPA Guidelines for Exposure to Naturally Occurring
Radioactive Materials, Evaluation of Guidelines for Exposures to Technologically Enhanced Naturally Occurring
Radioactive Materials, The National Academies Press, Washington, D.C., 1999.
55
U.S. EPA, Evaluation of EPA’s Guidelines for Technologically Enhanced Naturally Occurring Radioactive
Materials (TENORM)—Report to Congress (EPA 402-R-00-01) June 2000.
56
http://www.epa.gov/radiation/tenorm/regs.htm.
57
P.L. 109-58, 109th Cong., 1st Sess., 119 Stat. 594 (2005).
58
P.L. 109-58, § 65, 109th Cong., 1st Sess., 119 Stat. 807(2005).
59
Requirements for Expanded Definition of Byproduct Material; Proposed Rule, 71 Fed. Reg. 42951—42994 (July 28,
2006).
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other processes where radium-226 may be unintentionally concentrated.60 The specific example
of “residuals from treatment of water to meet drinking water standards” is given as a diffuse
source.
Recently, the Rocky Mountain Low-Level Radioactive Waste Compact’s authority to dispose of
NORM and TENORM has been called into question over the assertion that its jurisdiction
violates the Commerce Clause of the U.S. Constitution. Congress gave its consent to the Rocky
Mountain Low-Level Radioactive Waste Compact, consisting originally of the states of Arizona,
Colorado, Nevada, New Mexico, Utah, and Wyoming. 61 Arizona, Utah, and Wyoming later
withdrew from the Compact, leaving Colorado, Nevada, and New Mexico as remaining Compact
members.62 The Rocky Mountain Compact defines low-level waste as specifically excluding
radioactive waste generated by defense activities, high-level waste (from spent nuclear fuel
reprocessing), transuranic waste (produced from nuclear weapons fabrication), 11e(2) byproduct
material, 63 and mining process-related wastes.64 However, under Article VII(d) of the Compact,
both the Compact’s board and the host state may authorize management of any radioactive waste
other than low-level wastes upon consideration of various factors, such as the existence of
transuranic elements.65
A review of the legislative history of the Rocky Mountain Compact did not appear to reveal the
intent of Congress with respect to the specific responsibility of the states concerning NRCdefined A, B, and C class wastes. A statement in the legislative history of the Southeast Interstate
Compact, however, may provide an indication of Congress’s intent:
The definition of low-level waste in the compact may vary, but the compact provides for
adjustments and flexibility under its own procedures adequate to allow the compact to handle
waste for which the states are responsible.66
On the basis of the Compact’s Article VII and the language of H.Rept. 99-317, quoted above, that
accompanied H.R. 1267, it might be argued that the Compact’s jurisdiction extends to TENORM
when for disposal purposes TENORM meets the criteria of Class A, B, or C low-level radioactive
waste. Thus, the Compact’s authority to dispose of low-level radioactive waste would appear
restricted by the Energy Policy Act of 2005. TENORM that poses a threat similar to the threat
posed by a discrete source of radium-226 would arguably be outside the jurisdiction of the
Compact. A diffuse source of radium-226 (i.e., TENORM ) that does not pose a similar threat,
however, would appear to remain within the jurisdiction of the Compact’s Article VII(d)
provision.
60
Id., at 42959-42960.
P.L. 99-240, § 226, 99th Cong., 1st Sess., 99 Stat. 1902 (1985).
62
http://www.nrc.gov/waste/llw-disposal/compacts.html.
61
63
Section 11(e)2 of the Atomic Energy Act, 42 U.S.C. § 2014(e)(2), defines byproduct material to include the tailings
or wastes produced by extraction or concentration of uranium or thorium from any ore processed primarily for its
source content.
64
P.L. 99-240, § 226, Art. II(g), 99th Cong., 1st Sess., 99 Stat. 1903 (1985).
65
P.L. 99-240, § 226, Art. VII(d), 99th Cong., 1st Sess., 99 Stat. 1908 (1985).
66
H.R. REP. NO. 99-317, at 3 (1985).
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Uranium Mill Tailings
Uranium and thorium mill tailings are the waste byproducts of ore processed primarily for its
source material (i.e., uranium or thorium) content (10 C.F.R. 40.4). The tailings contain
radioactive uranium decay products and heavy metals. Mined ores are defined as source material
when containing 0.05 % or more by weight of uranium or thorium (10 C.F.R. 20.1003).
Byproduct material does not include underground ore bodies depleted by solution extraction.
Tailings or waste produced by the extraction or concentration of uranium or thorium is defined
under Section 11e.(2) of the Atomic Energy Act as amended by Title II of the Uranium Mill
Tailings Radiation Control Act of 1978 (UMTRCA , 42 U.S.C. 7901), and is simply referred to as
11e.(2) byproduct material. UMTRCA provided for stabilization and disposal of tailings to
mitigate the hazard of radon diffusion into the environment, and other hazards. Radon is a
daughter-product of uranium/thorium radioactive decay.
The NRC regulates the siting and design of tailings impoundments, disposal of tailings or wastes,
decommissioning of land and structures, groundwater protection standards, testing of the radon
emission rate from the impoundment cover, monitoring programs, airborne effluent and offsite
exposure limits, inspection of retention systems, financial surety requirements for
decommissioning and long-term surveillance and control of the tailings impoundment, and
eventual government ownership of pre-1978 tailings sites under an NRC general license.67
Waste Disposal Policy Issues
The AEC first acknowledged the problem of waste disposal in 1955. Concerned over the hazard
of radioactive waste, the AEC awarded a contract to the National Academy of Sciences to conduct
research on methods to dispose of radioactive waste in geologic media and recommend disposal
options within the continental limits of the United States.68 The Academy’s suggestion, at that
time, was that disposal in cavities mined out in salt beds or salt domes offered the most practical
and immediate solution.
In the mid-1960s, the AEC conducted engineering tests on disposing spent fuel in a salt mine near
Lyons, Kansas. After developing conceptual repository designs for the mine, AEC abandoned the
Lyons project in 1972 due to technical difficulties. The AEC went on to identify another site in a
salt deposit and announced plans for a retrievable surface storage program as an interim measure
until a repository could be developed, but the plan was later abandoned. 69
In the 1970s, the Energy Research and Development Administration (ERDA), and later the
Department of Energy (DOE), began a program of screening various geologic media for a
repository (including salt deposits), and the federal sites of the Hanford Reservation and Nevada
67
U.S. NRC, Appendix A to Part 40—Criteria Relating to the Operation of Uranium Mills and the Disposition of
Tailings or Wastes Produced by the Extraction or Concentration of Source Material from Ores Processed Primarily for
Their Source Material Content, at http://www.nrc.gov/reading-rm/doc-collections/cfr/part040/part040-appa.html.
68
Committee on Waste Disposal, National Research Council, The Disposal of Radioactive Waste on Land, National
Academies Press, Washington D.C., 1957.
69
Commission on Geosciences, Environment and Resources, Nuclear Wastes: Technologies for Separations and
Transmutation, National Academies Press, Washington D.C., 1996.
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Test Site. The national problem created by accumulating spent nuclear fuel and radioactive waste
prompted Congress to pass the Nuclear Waste Policy Act of 1982 (NWPA). The potential risks to
public health and safety required environmentally acceptable waste disposal solutions, and the
Act provided for developing repositories to dispose of high-level radioactive waste and spent
nuclear fuel. Under the Act, the Department of Energy will assume title to any high-level
radioactive waste or spent nuclear fuel accepted for a disposal in a repository constructed under
the Act (42 U.S.C. 10131).
In 2002, the President recommended approval of the Yucca Mountain repository site in Nevada.
In a recent district court ruling, however, EPA’s 10,000-year safety standard on radiation
containment at the site was found to be inconsistent with the congressionally mandated
recommendations of the National Academy of Sciences.70 Depending upon successful resolution
of the matter and the NRC’s granting a license, the repository could begin to accept high-level
waste and spent nuclear fuel in the next decade. The Energy Department intends to submit a
license application for Yucca Mountain in mid-2008.
The controversy over DOE waste incidental to reprocessing appears to have been resolved by
redefining high-level radioactive wastes as excluding the residue in high-level waste storagetanks. However, Congress has requested the National Research Council to study DOE’s plans to
manage the residual tank waste and report on the adequacy of the plans (P.L. 108-375). The DOE
also operates the Waste Isolation Pilot Plant in New Mexico to dispose of the transuranic waste
generated by the weapons program. New Mexico’s Governor, concerned that waste incidental to
reprocessing could end up at WIPP, ordered the state’s Department of Environmental
Management to amend WIPP’s hazardous waste permit so that only waste listed on DOE’s
Transuranic Waste Baseline Report is explicitly permitted for disposal at WIPP.71
When Congress passed the Low-Level Radioactive Waste Policy Act in 1980, three states—
Nevada, South Carolina, and Washington—hosted disposal sites for commercially generated lowlevel waste. The Act encouraged the formation of multi-state compacts in which one state would
host a disposal facility for the member states. The new facilities were to begin operation in by the
end of 1985. When it became clear that the deadline would not be met, Congress extended the
deadline to the end of 1992 in the amended Act of 1986 (P.L. 99-240). Since then, a new
commercial site has been licensed in Utah, and the Nevada site has closed.
Much of the low-level waste disposed of as Class A consists of debris, rubble, and contaminated
soil from decommissioning DOE and commercial nuclear facilities that contain relatively little
radioactivity. These decommissioning wastes make up much larger volumes than low-level waste
generated by operating nuclear facilities. The term “low-activity” has been used in describing the
waste, although it lacks regulatory or statutory meaning. The National Research Council, in its
interim report Improving the Regulation and Management of Low-Level Radioactive Wastes
found that the current system of regulating low-activity waste lacked overall consistency.72 As a
70
Nuclear Energy Institute, Inc. V. Environmental Protection Agency, No. 1258 United States Court of Appeals, July
9, 2004.
71
New Mexico Environmental Department, NMED WIPP Information Page, at http://www.nmenv.state.nm.us/wipp/.
72
National Research Council of the National Academies, Improving the Regulation and Management of Low-Level
Radioactive Wastes—Interim Report on Current Regulations, Inventories, and Practices, National Academies Press,
2003.
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consequence, waste streams having similar physical, chemical, and radiological characteristics
may be regulated by different authorities and managed in disparate ways.
In an Advance Notice of Proposed Rulemaking (ANPR), the EPA proposed analyzing the
feasibility of disposing of certain low-activity radioactive wastes in the RCRA Subtitle C
(hazardous waste) landfills, provided that legal and regulatory issues can be resolved. 73 The NRC,
in collaboration with the state of Michigan, recently permitted certain very low-activity wastes
from decommissioning of the Big Rock Point nuclear power plant to be sent to a RCRA Subtitle
D (solid waste) landfill, and other states have also determined that solid waste landfills offer
sufficient protection for low-activity waste. 74 In a recent decision, however, the NRC rejected a
staff proposal to permanently allow disposal of low-activity waste in solid waste landfills.75 If
found to be acceptable, disposing of low-activity waste at RCRA C and D landfills could alleviate
the future capacity constraints at the three operating low-level waste facilities.
Radioactive waste classification continues to raises issues for policymakers. Radioactive waste
generation, storage, transportation, and disposal leave little of the national geography unaffected.
The weapons facilities that processed and stored radioactive waste have left a lasting and
expensive environmental legacy that the DOE is attempting to remedy by accelerating the
cleanup of those contaminated sites. The standards for public exposure to low-level radiation
from the repository or cleanup of the weapons facilities have not been reconciled by EPA and
NRC. The lower limit on what may be classified as radioactive waste is undefined, and both EPA
and NRC jurisdiction overlap on disposal of this waste stream.
Glossary
BWR
boiling water reactor.
curie
the basic unit describing the radioactive intensity of a material. One curie equals
37 billion (37 x 109) disintegrations/second, which is approximately the activity
of 1 gram of radium.
isotope
one of several nuclides of the same element, thus the same number of protons
in the nucleus (e.g. 92 for uranium) but differing in the number of neutrons,
hence U-234, U-235, U-238.
microcurie
one millionth of a curie (1 x 10-6 curie); also expressed as µcurie
millicurie
one thousandth of a curie (1 x 10-3 curie); also expressed as mcurie
millirem
one-thousandth of a REM (Radiation Equivalent Man). It is the term for the
conventional unit of ionizing radiation dose (rad) equivalent used for radiation
protection purposes.
MTHM
metric ton of heavy metal. 1000 kilograms (the U.S. equivalent of 2,200 lbs) of
original uranium in fuel, excluding cladding and assembly hardware.
nanocurie
one billionth of a curie (1 x 10-9 curie); also expressed as ηcurie.
picocurie
one trillionth curie (1 x 10-12 curie); also expressed as pcurie.
73
68 Federal Register 65,120, November 18, 2003.
74
Margaret V. Federline , U.S. NRC, Management and Disposal Strategies for Low-Activity Waste in the U.S., White
Paper, December 8, 2004.
75
“NRC Surprises, Rejects Rule on Nuke Material Recycling and Disposal,” The Energy Daily, June 6, 2005
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PWR
pressurized water reactor.
Transuranic elements
neptunium, plutonium, americium, and curium.
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Appendix.
Table A-1. Uranium Mill Tailing Site Volume and Activity
Disposal Cell
Waste Volume
Disposal Cell
Radioactivity
Tailings
Activity
Site
Million
Cubic Yards
Million Cubic
Meters
Total Curies
(226Ra)
Average
Curies/
Cu. mtr.
Average
Curies/gram
(226Ra)
Maybell Mill Site, CO
3.50
4.58
445
0.0000972
0.000000000200
Mexican Hat Mill Site,
UT
3.48
4.55
1,800
0.0000978
0.000000000667
Edgemont Mill Site, SD
3.00
3.92
527
0.0001340
NA
Falls City Mill Site, TX
5.80
7.59
1,277
0.0001680
0.000000000189
Ambrosia Lake Mill
Site, NM
5.20
6.80
1,850
0.0002720
0.000000000571
Durango Mill Site, CO
2.53
3.31
1,400
0.0004530
0.000000000671
Rifle Mills (Old &
New) Mill Sites, CO
3.76
4.92
2,738
0.0005570
0.000000000760
Salt Lake City Mill Site,
UT
2.80
3.66
1,550
0.0007480
0.000000000481
Source: U.S. DOE Energy Information Administration; “Remediation of UMTRCA Title I Uranium Mill Sites
Under the UMTRA Project Summary Table: Uranium Ore Processed, Disposal Cell Material, and Cost for
Remediation as of December 31, 1999,” at http://www.eia.doe.gov/cneaf/nuclear/page/umtra/title1sum.html.
Notes: Total Curies and Average Curies expressed as Radium-226 equivalence; 1 cubic meter = 1.308 cubic
yards.
Table A-2. Low-Level Waste Commercial Disposal Site Volume and Activity
Site
Cubic Feet
Cubic Meter
Activity Curies
Curies/
cubic-meter
Barnwell, SC
788,000
22,316
443,600
19.88
Richland, WA
295,300
8,363
92,980
11.12
Beatty, NV
59,480
1,684
11,320
6.72
1 ft3 = 0.02832 m3
Source: U.S. DOE, Table 1. Commercial Gross Volume and Activity Distribution in Disposal of Low-Level and
Mixed Low-Level Radioactive Waste During 1990 (DOE/EH-0332p), August 1993.
Table A-3. Spent Fuel Specific Activity
Fuel Rod Type
BWRa
PWRb
PWRc
PWRd
PWRe
PWRf
Fuel Rod array
8x8
17x17
17x17
17x17
17x17
17x17
GW/d/MTHM
40
50
20
20
50
50
Congressional Research Service
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Radioactive Waste Streams: Waste Classification for Disposal
Fuel Rod Type
BWRa
PWRb
PWRc
PWRd
PWRe
PWRf
U-236 enrichment (%)
3.5
4.3
3
3
4.5
4.5
Decay time (years)
14
15
10
100
10
100
Activity / assembly (curies)
229594
68273
150000
20000
450000
40000
Nom vol/ assembly (cu. m)g
0.086
0.19
0.19
0.19
0.19
0.19
2669698
359332
789000
105000
2370000
211000
Calculated curies/ cu. M
Sources:
a.
Boiling Water Reactor, Appendix A, Table A-13, Yucca Mt. EIS
b.
Pressurized Water Reactor, Appendix A, Table A-12, Yucca Mt. EIS
c.
Pressurized Water Reactor, Appendix C, P 82, Oak Ridge National Laboratory “Investigation of Nuclide
Importance to Functional Requirements Related to Transport and Long-Term Storage of LWR Spent Fuel
(ORNL/TM/12742), 1995.
d.
Appendix C, P 82, ORNL/TM/12742.
e.
Appendix C, P 85, ORNL/TM12742.
f.
Appendix C, P 85, ORNL/TM12742.
g.
Table A-18, Reference Characteristics for Average Commercial Spent Fuel Assemblies, Appendix A,
Inventory of Characteristics of Spent Nuclear fuel, High-Level Radioactive Waste, and Other Materials,
Yucca Mountain EIS.
Notes: A typical fuel rod used in commercial nuclear power reactors consists of uranium dioxide pellets
surrounded by zirconium alloy cladding. The uranium oxide pellets consist of 3-4% fissionable uranium-235, and a
balance of nonfissionable U-238. An individual fuel assembly consists of arrays of fuel rods. The Energy
Information Administration (EIA) notes 131 reactor fuel assembly types on its Nuclear Fuel Data Survey Form
RW-859 (OMB No. 1901-0287). The assemblies range in weight from ~70 kilograms uranium for a Humboldt
Bay Assembly Class (boiling water reactor) to ~ 464 kilograms uranium for a Babcock & Wilcox 15 x 15
Assembly Class (pressurized water reactor). During the sustained chain reaction in an operating reactor, the U235 splits into highly radioactive fission products, while the U-238 is partially converted to plutonium-239 by
neutron capture, some of which also fissions. Further neutron capture creates other transuranic elements.
Congressional Research Service
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Radioactive Waste Streams: Waste Classification for Disposal
Figure A-1. 10 CFR 61.55 Table 1
Figure A-2. 10 CFR 61.55 Table 2
Congressional Research Service
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Radioactive Waste Streams: Waste Classification for Disposal
Author Contact Information
(name redacted)
Specialist in Energy and Energy Infrastructure
Policy
[redacted]@crs.loc.gov, 7-....
Congressional Research Service
34
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